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129] For mixtures of particles with z = 0 and z = 1, the conductivity was reported to be proportional to the product [MPC0 ][MPC+ ] and goes through a maximum when these concentrations are equal. [129] This quantised double layer charging is due to Coulomb blockade, which gives rise to periodic metal-insulator transitions at integer values of the average charge state of the particles. [132,133] Thus far, all reported data on Coulomb blockade in MPC films has been obtained using techniques where an electrical connection to the film is a prerequisite to measuring the conductivity.

E. Roitberg, and J. L. Krause, Physical Review Letters, 2004, 92(15), 158301/1–158301/4. [68] W. Haiss, H. V. Zalinge, S. J. Higgins, D. Bethell, H. Hoebenreich, D. J. Schiffrin, and R. J. Nichols, Journal of the American Chemical Society, 2003, 125(50), 15294–15295. [69] Y. Tanaka, A. Inagaki, and M. Akita, Chemical Communications (Cambridge, United Kingdom), 2007, (11), 1169–1171. [70] H. -Q. Lu, Physics Letters A, 2007, 371, 465–468. [71] Y. Y. Liang, F. Jiang, Y. X. Zhou, H. Chen, R. Note, H.

N. Paddon-Row, Accounts of Chemical Research, 1994, 27(1), 18–25. [66] C. Zhang, Y. -P. Cheng, Y. Xue, M. A. Ratner, X. G. Zhang, and P. Krstic, Physical Review B: Condensed Matter and Materials Physics, 2006, 73(12), 125445/1–125445/5. [67] C. Zhang, M. H. Du, H. P. Cheng, X. G. Zhang, A. E. Roitberg, and J. L. Krause, Physical Review Letters, 2004, 92(15), 158301/1–158301/4. [68] W. Haiss, H. V. Zalinge, S. J. Higgins, D. Bethell, H. Hoebenreich, D. J. Schiffrin, and R. J. Nichols, Journal of the American Chemical Society, 2003, 125(50), 15294–15295.

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