By R. R. Dogonadze, A. M. Kuznetsov (auth.), Brian E. Conway, John O’M. Bockris, Ernest Yeager, Shahed U. M. Khan, Ralph E. White (eds.)
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Extra resources for Comprehensive Treatise of Electrochemistry: Volume 7 Kinetics and Mechanisms of Electrode Processes
38) related to the change of the proton state is temperature independent and is equal to the Franck-Condon factor for the ground initial and final proton vibrational states: s =
Chem. 72, 891 (1968). 38. V. G. Levich, R. R. Dogonadze, E. D. German, A. M. Kuznetsov, and Yu. I. Kharkats, Electrochim. Acta 15,353 (1970). 39. E. D. German, R. R. Dogonadze, A. M. Kuznetsov, V. G. Levich, and Yu. I. Kharkats, Elektrokhimiya 6, 350 (1970). 40. R. A. Marcus, Ann. Rev. Phys. Chem. 15, 155 (1964). 41. V. G. Levich, in Advanced Treatise of Physical Chemistry, Vol. 9B, H. Eyring, D. Henderson, and J. , Academic Press, New York (1970), p. 986. 42. R. R. Dogonadze, in Reactions of Molecules at Electrodes, N.
RN) + UAr) (59) where U(rh . , rN) is the interaction energy of all the ions except a given reacting one. It includes the interaction of the ions and their "images" with one another, and with the electrode, and does not depend on the coordinate of the reacting ion, r. U z (r) is the energy of interaction of the reacting ion, A Z, with its unscreened self-image in the electrode, Vi(r, rl' ... , rN) is the energy of the interaction of the reacting ion A z with the other ions and their images and with the electric field of the electrode; Q i is the statistical sum of the ionic system in the initial state.